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电化学(中英文) ›› 2017, Vol. 23 ›› Issue (2): 102-109.  doi: 10.13208/j.electrochem.161244

• 田昭武先生90大寿祝贺专辑(厦门大学 孙世刚 林昌健教授主编) • 上一篇    下一篇

Pt-skin的Pt基双金属电催化的氧还原设计

张斌伟, 王云晓, 徐燕斐, 刘华坤, 窦士学*   

  1. 超导电子材料研究所,澳大利亚创新材料研究所,伍伦贡大学,创新校区,澳大利亚新南威尔士州,北卧龙岗,2500
  • 收稿日期:2016-12-08 修回日期:2017-01-19 出版日期:2017-04-28 发布日期:2017-01-29
  • 通讯作者: 窦士学 E-mail:Shi@uow.edu.au
  • 基金资助:

    This work is supported by Australian Research Council (ARC) (LP120200432 and DP140104062), Baosteel-Australia joint research and development center (Baosteel Grant no. BA14006), and the Commonwealth of Australia through the Automotive Australia 2020 Cooperative Research Centre (Auto CRC)

Designing Pt-skin of Pt-based Bimetallic electrocatalysts for Oxygen Reduction Reaction

Binwei Zhang, Yunxiao Wang, Yanfei Xu, Huakun Liu, Shixue Dou*   

  1. Institute for Superconducting and Electronic Materials, Australian Institute of Innovative Materials, University of Wollongong, Innovation Campus, Squires Way, North Wollongong, New South Wales 2500, Australia.
  • Received:2016-12-08 Revised:2017-01-19 Published:2017-04-28 Online:2017-01-29
  • Contact: DOU Shi-Xue E-mail:Shi@uow.edu.au
  • Supported by:

    This work is supported by Australian Research Council (ARC) (LP120200432 and DP140104062), Baosteel-Australia joint research and development center (Baosteel Grant no. BA14006), and the Commonwealth of Australia through the Automotive Australia 2020 Cooperative Research Centre (Auto CRC)

摘要:

过去几十年,能源储存转化领域取得重大的进展. 而Pt-skin的Pt基双金属电催化剂在调控电催化剂的电子结构具有巨大的前景,特别是对于氧还原反应而言. 本工作主要综述了最近几年关于Pt-skin的Pt 基双金属电催化剂的设计制备,以及其性能. 本文的主要重点在于系统的综述了Pt-skin的Pt 基双金属电催化剂的合成方法,以及其对于氧还原反应的机理研究.

关键词: Pt, 双金属, 电催化剂, 氧还原

Abstract:

In the past decade, great advancement has been made in the development of nanocatalysts for energy conversion and storage. Pt-skin of Pt-based bimetallic has shown a great potential in the tuning the electronic structures of electrocatalytically active materials toward oxygen reduction reaction. Here, we offer a brief overview of the recent research on the design and preparation of catalysts. Our focus is paid on the systematic studies of preparation and performance of Pt-skin catalysts towards oxygen reduction reaction.

Key words: Pt, bimetallic, electrocatalysts, oxygen reduction reaction

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