影响电池性能的因素：金属离子溶剂化结构衍生的界面行为还是固体电解质界面膜?
收稿日期: 2022-10-06
修回日期: 2022-10-19
网络出版日期: 2022-11-28
Which Factor Dominates Battery Performance: Metal Ion Solvation Structure-Derived Interfacial Behavior or Solid Electrolyte Interphase Layer?
Received date: 2022-10-06
Revised date: 2022-10-19
Online published: 2022-11-28
程浩然 , 马征 , 郭营军 , 孙春胜 , 李茜 , 明军 . 影响电池性能的因素：金属离子溶剂化结构衍生的界面行为还是固体电解质界面膜?[J]. 电化学, 2022 , 28(11) : 2219012 . DOI: 10.13208/j.electrochem.2219012
Solid-electrolyte interphase (SEI) layer formed on the electrode by electrolyte decomposition has been considered to be one of the most important factors affecting the battery performance. We discover that the metal ion solvation structure can also influence the performance, particularly, it can elucidate many phenomena that the SEI cannot. In this review, we summarize the importance of the metal ion solvation structure and the derived metal ion de-solvation behaviors, by which we can build an interfacial model to show the relationship between the interfacial behavior and electrode performance, and then apply to different electrode and battery systems. We emphasize the influences of ionic and molecular interactions on electrode surface that differ from previous SEI-based interpretations. This review provides a new view angle to understand the battery performance and guide the electrolyte design.
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