基于流动池的电化学二氧化碳还原研究进展
收稿日期: 2020-05-05
修回日期: 2020-05-20
网络出版日期: 2020-07-06
基金资助
国家科技部基金项目(2017YFA0204800);国家自然科学基金项目资助(2190020225)
Electrochemical Carbon Dioxide Reduction in Flow Cells
Received date: 2020-05-05
Revised date: 2020-05-20
Online published: 2020-07-06
范佳 , 韩娜 , 李彦光 . 基于流动池的电化学二氧化碳还原研究进展[J]. 电化学, 2020 , 26(4) : 510 -520 . DOI: 10.13208/j.electrochem.200443
Electrochemical carbon dioxide reduction (CO2RR) is an appealing approach to convert atmospheric CO2 to value-added fuels and industrial chemicals, and may play an important role during the transition to a carbon-neutral economy. In order to make this technology commercially viable, it is essential to pursue CO2RR in flow reactors instead of conventional H-type reactors, and to combine electrocatalyst development with system engineering. In this review, we overview the cell configurations and performance advantages of the two types of flow reactors, analyze their shortcomings, and discuss the effects of their different components including gas diffusion electrode and ion exchange membrane. A brief perspective is offered at the end for the possible future research directions in this emerging field.
Key words: CO2 reduction; electrocatalysis; flow cell; current density
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