水溶液中二氧化碳电还原技术的发展现状、挑战及对策
收稿日期: 2018-10-05
修回日期: 2018-11-10
网络出版日期: 2019-08-28
基金资助
上海市科学技术委员会国际科技合作项目(No. 18160723600)和广西科研与技术开发计划项目(No. GUIKE AD17195084)资助
Statuses, Challenges and Strategies in the Development of Low-Temperature Carbon Dioxide Electroreduction Technology
Received date: 2018-10-05
Revised date: 2018-11-10
Online published: 2019-08-28
张旭锐 , 邵晓琳 , 易 金 , 刘予宇 , 张久俊 . 水溶液中二氧化碳电还原技术的发展现状、挑战及对策[J]. 电化学, 2019 , 25(4) : 413 -425 . DOI: 10.13208/j.electrochem.180943
Low-temperature carbon dioxide (CO2) electrochemical reduction technology is a hotspot for research and development in recent years as a way to reduce the negative impact of CO2 on the environment and to generate energy storage through converting electricity to low-carbon fuels. Although basic research on catalyst activity, product selectivity, and reaction mechanism has been widely reported, the design and practicality of catalytic stability and corresponding electrochemical reactor systems have not been given sufficient attention and systematic development. In this paper, two important factors affecting the development of CO2 electrochemical reduction technology in low temperature aqueous solution (catalyst and reaction system developments) are summarized. From the perspective of technical application requirements and based on the current research and development status, the main challenges are discussed. Some suggestions for future research directions are suggested to overcome the challenges.
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