直接乙醇燃料电池阳极电催化剂的设计与优化：C-C键活化及C1途径选择性调控的研究进展与挑战

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秦愷池^a, 霍孟田^a, 梁宇^a, 朱思远^b, 邢子豪^a^,^*(

), 常进法^a^,^*(

)

Design and Optimization of Anode Catalysts for Direct Ethanol Fuel Cells: Advances and Challenges in C-C bond Activation and Selective Modulation of the C1 Pathway

Qin Kai-Chi^a, Huo Meng-Tian^a, Liang Yu^a, Zhu Si-Yuan^b, Xing Zi-Hao^a^,^*(

), Chang Jin-Fa^a^,^*(

)

Fig 12.. (A) DOS plots and free energy diagrams of EOR-related adsorption on Rh(111) and RhBi(111) surfaces. Reproduced with permission of Ref. [110]. Copyright 2023, Elsevier. (B) The k3-weighted Rh K-edge EXAFS spectra of Rh_atO-Pt NCs/C and Rh_clO-Pt NCs/C. Reproduced with permission of Ref. [119]. Copyright 2022, Washington, DC. (C) Schematic reaction mechanism of ethanol electrooxidation on 0.2SnO₂-Rh NSs/C. Reproduced with permission of Ref. [120]. Copyright 2020, Wiley-VCH. (D) Scheme of Rh/Rh-M NSs. Reproduced with permission of Ref. [121]. Copyright 2022, Elsevier.