固态电解质反应器驱动的大气环境CO2捕集与电催化转化

华炎波, 倪宝鑫, 蒋昆

Ambient CO2 Capture and Valorization Enabled by Tandem Electrolysis Using Solid-State Electrolyte Reactor

Yan-Bo Hua, Bao-Xin Ni, Kun Jiang

Figure 4. CO2RR enabled by SSE. a, the SSE configuration for HCOOH synthesis and the HCOOH FE under different cell voltage [42]. Reproduced with permission of Ref. [42]. Copyright 2019, Springer Nature. b, the I-V curve of Pb1Cu catalyst during SSE electrolysis (inset: TEM image of the catalyst) [62]. Reproduced with permission of Ref. [62]. Copyright 2021, Springer Nature. c, a 40-cm2 SSE set up for continuous production of 2.5 mol·L-1 HCOOH [63]. Reproduced with permission of Ref. [63]. Copyright 2024, National Academy of Sciences. d, the energy efficiency and HCOOH concentration under series of cell voltage with the energy flow diagram coupling with biosynthesize [64]. Reproduced with permission of Ref. [64]. Copyright 2021, Springer Nature. e, a tandem system combing electrochemical CO2 capture and conversion from simulated flue gas [65]. Reproduced with permission of Ref. [65]. Copyright 2025, American Chemical Society.